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Updated: Jun 18, 2025

Quantifying X-Ray Fluorescence Data Using MAPS
Published on: February 17, 2018
Machine learning based unfolding of x-ray spectra from filter stack spectrometer data
M Alvarado Alvarez1, B T Wolfe1, C-S Wong1
1Los Alamos National Laboratory, Los Alamos, New Mexico 87545, USA.
Neural networks accurately unfold X-ray spectra from filter stack spectrometers. This method shows robustness to errors and potential for high-repetition-rate applications.
Area of Science:
- Spectroscopy
- Machine Learning
- X-ray Physics
Background:
- Filter stack spectrometers measure X-ray energy deposition via photo-stimulated luminescence (PSL).
- Accurate X-ray spectra unfolding is crucial for various scientific and industrial applications.
Purpose of the Study:
- To apply neural networks for X-ray spectra unfolding using filter stack spectrometer data.
- To evaluate the accuracy, robustness, and speed of the neural network approach.
Main Methods:
- Training a neural network on synthetic X-ray data (<1 MeV) with Maxwellian and Gaussian distributions.
- Utilizing PSL measurements from five distinct filter stack spectrometer designs.
- Testing the network's performance against ground truth spectra and simulated experimental errors.
Main Results:
- Neural network predictions closely matched ground truth spectra for single distributions, with <20% difference at high energies.
- The network demonstrated robustness to experimental errors (<5%) and some ability to unfold mixed distributions.
- Unfolding rates exceeded 1 Hz, suitable for high-repetition-rate systems.
Conclusions:
- Neural networks offer a powerful and efficient tool for X-ray spectra unfolding with filter stack spectrometers.
- The developed method is accurate, robust to experimental noise, and fast enough for demanding applications.
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