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Screening the organic materials database for superconducting metal-organic frameworks.

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Researchers explored metal-organic frameworks as green alternatives to inorganic materials. They identified a promising candidate, C9H8Mn2O11, exhibiting superconductivity at temperatures below 100mK.

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Area of Science:

  • Materials Science
  • Condensed Matter Physics
  • Green Chemistry

Background:

  • Rising costs and environmental impact of inorganic materials drive demand for sustainable alternatives.
  • Organic compounds often have complex structures hindering rapid property screening.
  • Metal-organic frameworks (MOFs) offer a potential class of 'green' functional materials.

Purpose of the Study:

  • To overcome the challenge of screening complex organic materials for functional properties.
  • To identify potential superconducting candidates within the metal-organic-frameworks organic materials database.
  • To investigate the electron-phonon coupling in MOFs as a proxy for superconductivity.

Main Methods:

  • Utilized a recently proposed proxy for electron-phonon coupling for high-throughput screening.
  • Screened a database of metal-organic-frameworks for superconducting properties.
  • Isolated and performed in-depth analysis on the most promising candidate material.

Main Results:

  • Identified several potential superconducting candidates among MOFs.
  • The material C9H8Mn2O11 emerged as the most promising candidate.
  • Experimental evidence indicates superconductivity in C9H8Mn2O11 below 100 millikelvin (mK).

Conclusions:

  • Metal-organic frameworks are viable candidates for discovering novel superconducting materials.
  • The developed screening proxy effectively identifies potential superconductors in complex organic structures.
  • C9H8Mn2O11 represents a significant finding in the search for green superconductors.