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Development of Thermoplastic Bi-Component Electrodes for Triboelectric Impact Detection in Smart Textile Applications
David Seixas Esteves1,2, Amanda Melo2, Bruno Peliteiro2
1Department of Mechanical Engineering, Faculty of Engineering, University of Porto, 4200-465 Porto, Portugal.
Polymers
|January 25, 2025
Summary
Researchers developed a flexible, conductive composite for smart textiles using multi-walled carbon nanotubes (MWCNTs) and thermoplastic elastomer (TPE) in a polypropylene (PP) matrix. This material enables advanced triboelectric sensors for impact detection and motion tracking in wearable technology.
Area of Science:
- Materials Science
- Polymer Science
- Textile Engineering
Background:
- Smart textiles require materials balancing traditional textile properties with electronic functionality.
- Developing flexible, conductive composites is crucial for integrating electronics into textiles for wearable applications.
Purpose of the Study:
- To create a flexible, electrically conductive composite material for sensor electrodes using a bi-component extrusion process.
- To optimize the composite composition for conductivity, flexibility, and processability in a polypropylene matrix.
Main Methods:
- Fabrication of a composite core using multi-walled carbon nanotubes (MWCNTs), polypropylene (PP), and thermoplastic elastomer (TPE) via bi-component extrusion.
- Optimization of MWCNT (2.5-10 wt.%) and TPE (0-50 wt.%) content within the PP matrix.
- Lamination of the optimized composite filament (5 wt.% MWCNT/PP/25 wt.% TPE core with TPE sheath) into a textile triboelectric sensor.
Main Results:
- Significant decrease in electrical resistivity observed between 2.5 and 5 wt.% MWCNT, with resistivity ranging from 7.64 ± 4.03 x 10^4 to 1.15 ± 0.10 x 10^-1 Ω·m.
- Incorporating 25 wt.% TPE enhanced composite flexibility without significantly compromising mechanical properties or processability.
- The developed triboelectric sensor demonstrated a peak-to-peak output voltage of approximately 5 V per filament and 15 V with five filaments under a 100 N force.
Conclusions:
- An innovative flexible conductive composite material was successfully developed for smart textile applications.
- The composite material is suitable for fabricating triboelectric sensor electrodes with potential for impact detection, fall monitoring, and motion tracking.
- The study highlights the successful integration of advanced materials and processing techniques for next-generation wearable technology.

