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Dynamic Pore-scale Reservoir-condition Imaging of Reaction in Carbonates Using Synchrotron Fast Tomography
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Robust broadband ptychography algorithms for high-harmonic soft X-ray supercontinua.

Benjamin Shearer, Henry Kapteyn, Iona Binnie

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    This summary is machine-generated.

    We developed PaCMAN, a ptychography algorithm for high-quality imaging with broadband light sources, reducing noise and improving accuracy. This method enables faster, lower-dose imaging for sensitive materials and advanced applications.

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    Area of Science:

    • Coherent diffractive imaging
    • Computational imaging
    • Soft X-ray microscopy

    Background:

    • Ptychography is a powerful lensless imaging technique.
    • Existing methods struggle with broadband illumination and various noise sources.
    • Monochromatization improves accuracy but is limited for discrete spectra.

    Purpose of the Study:

    • To introduce PaCMAN, a novel ptychography algorithm for high-quality imaging.
    • To enhance accuracy with broadband sources and noise robustness.
    • To develop a multi-spectral variant (Ms. PaCMAN) and compare performance.

    Main Methods:

    • Demonstration of PaCMAN with broadband illumination.
    • Extension of monochromatization techniques for discrete spectra.
    • Conversion of PaCMAN to a multi-spectral variant (Ms. PaCMAN).
    • Comparison of speed- and dose-optimized PaCMAN against ePIE.

    Main Results:

    • PaCMAN reconstructs high-quality images with broadband sources, robust to noise.
    • Ms. PaCMAN outperforms multi-spectral ePIE.
    • Speed-optimized PaCMAN achieves high quality 4x faster than ePIE.
    • Dose-optimized PaCMAN requires 1.5-2x less dose than ePIE.

    Conclusions:

    • PaCMAN enables rapid sub-10 nm imaging with soft X-ray supercontinua.
    • The algorithm advances attosecond coherent diffractive imaging.
    • PaCMAN significantly reduces radiation dose for imaging sensitive materials.