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Updated: May 15, 2025

Measurement of Scattering Nonlinearities from a Single Plasmonic Nanoparticle
Published on: January 3, 2016
Localization of nanoscale objects with light singularities
Thomas A Grant1, Anton N Vetlugin2, Eric Plum1
1Optoelectronics Research Centre, University of Southampton, Southampton, SO17 1BJ, UK.
Abstract:
Unprecedented atomic-scale measurement resolution has recently been demonstrated in single-shot optical localization measurements based on deep-learning analyses of diffraction patterns of topologically structured light scattered from objects. Here, we show that variations in the diffraction patterns caused by positional changes of an object depend upon the spatial derivatives of the amplitude and phase of the incident field, most strongly around phase singularities. Despite lower intensity near the singularity, an orders-of-magnitude increase in Fisher information contained in the diffraction patterns can be achieved when a nano-object is illuminated by light containing phase singularities, rather than a plane wave. Our work provides a fundamental explanation and motivation for singularity-based metrology with deeply subwavelength precision.

