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Published on: March 24, 2019
Image-Potential States on a 2D Gr-Ferromagnet Hybrid: Enhancing Spin and Stacking Sensing.
Maciej Bazarnik1,2, Anika Schlenhoff1,2
1Institute of Physics, University of Münster, D-48149 Münster, Germany.
Image-potential states on graphene/iron/iridium reveal spin polarization variations across moiré unit cells. This technique offers new insights into buried interfaces in 2D hybrid materials.
Area of Science:
- Surface Science
- Condensed Matter Physics
- Materials Science
Background:
- Graphene on metals like Fe/Ir(111) forms moiré superlattices influencing electronic properties.
- Image-potential states are sensitive probes of surface and interface electronic structure.
Purpose of the Study:
- Investigate spin-resolved properties of image-potential states on Gr/Fe/Ir(111).
- Determine sensitivity to interfacial structure and spin transfer.
- Explore potential for imaging buried interface magnetism.
Main Methods:
- Spin-resolved scanning tunneling microscopy (SR-STM).
- Spin-resolved scanning tunneling spectroscopy (SR-STS).
- Resonant tunneling topography and spectroscopy.
Main Results:
- Image-potential states show sensitivity to graphene-Fe distance and interfacial spin transfer.
- Stacking contrast (fcc vs. hcp sites) is observed in image-potential states, unlike direct tunneling.
- Site- and energy-dependent spin polarization of image-potential states is mapped across the moiré unit cell.
- Lowest image-potential states on on-top sites exhibit high spin polarization, reflecting buried interface spin density.
Conclusions:
- Image-potential states provide a unique contrast mechanism for buried interfaces.
- SR-STM/STS of image-potential states can image structural, electronic, and magnetic properties simultaneously.
- This method is valuable for studying 2D hybrid materials and heterostructures with buried interfaces.
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