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mJ-level 7-octave ultraflat white laser encompassing 200-25,000 nm.

Lihong Hong1,2,3, Renyu Feng2, Yuanyuan Liu1

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Researchers developed an intense ultrafast white laser spanning deep-ultraviolet to far-infrared wavelengths. This novel laser enables full-spectrum spectroscopy for diverse scientific and technological applications.

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Area of Science:

  • Laser Physics
  • Spectroscopy
  • Nonlinear Optics

Background:

  • Ultrafast laser technology is crucial for advanced spectroscopy.
  • Broadband laser sources are needed for comprehensive material analysis.
  • Current limitations exist in achieving continuous spectral coverage from DUV to FIR.

Purpose of the Study:

  • To create an intense ultrafast white laser with continuous spectral coverage from deep-ultraviolet (DUV) to far-infrared (FIR).
  • To demonstrate the laser's capability for full-spectrum laser spectroscopy.
  • To explore applications in basic science and technology.

Main Methods:

  • Utilized synergic nonlinear up-conversion and down-conversion modules.
  • Employed a mid-infrared (MIR) seed pulse laser generated via optical-parametric chirped pulse amplification and krypton gas-filled hollow-core fiber.
  • Designed a chirped-periodic poling lithium niobate (CPPLN) crystal for second-order nonlinear harmonic generation and AgGaSe2 crystals for difference-frequency generation.

Main Results:

  • Achieved an intense white laser with 200-25,000 nm bandwidth and ~1 mJ pulse energy.
  • Generated DUV wavelengths down to 200 nm with ~40% conversion efficiency.
  • Produced MIR-FIR laser wavelengths from 2000-25,000 nm with an overall 18% conversion efficiency.

Conclusions:

  • The developed 7-octave ultraflat DUV-FIR white laser provides unprecedented power for simultaneous probing of electronic, vibrational, and lattice dynamics.
  • This technology opens new avenues for full-spectrum laser spectroscopy.
  • Potential applications span a wide range of physical, chemical, and biological substances and processes.