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Spatial Correlations of Charge Density Wave Order across the Transition in 2H-NbSe_{2}
Seokjo Hong1, Jaewhan Oh1, Jemin Park1
1Korea Advanced Institute of Science and Technology (KAIST), Department of Physics, Daejeon 34141, Republic of Korea.
None:
Charge density waves (CDWs) involve coupled amplitude and phase degrees of freedom, but direct access to local amplitude correlations remains experimentally challenging. Here, we report cryogenic four-dimensional scanning transmission electron microscopy measurements of CDW ordering in a 2H-NbSe_{2} flake of 24 nm thickness, enabled by liquid-helium-based cooling. By mapping the spatial distribution of CDW superlattice intensities at nanometer-scale resolution and analyzing their autocorrelations, we extract the temperature-dependent correlation length associated with the local amplitude of the CDW order parameter, independent of global phase coherence. Our results reveal that a finite local CDW amplitude is already established well above the transition temperature. When the system is cooled below the transition temperature down to 20 K, the correlation length extends to nearly 110 nm, and the local CDW amplitude is found to strongly anticorrelate with the local strain field.
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