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Ultrafast Laser-Driven Asymmetric Demagnetization Dynamics in d-Wave Altermagnets
1School of Physics, State Key Laboratory of Electronic Thin Films and Integrated Devices, University of Electronic Science and Technology of China, Chengdu 611731, China.
Altermagnets exhibit ultrafast spin manipulation. Laser polarization selectively excites spin transfer in V2Se2O crystals, generating net magnetization, with lower dimensionality enhancing this effect for spintronic applications.
Area of Science:
- Condensed Matter Physics
- Materials Science
- Quantum Mechanics
Background:
- Altermagnetism (AM) is an unconventional spin-ordered phase offering potential for ultrafast spin manipulation.
- Understanding laser-driven spin dynamics in low-dimensional altermagnets is crucial but remains unclear.
Purpose of the Study:
- Investigate laser-induced spin dynamics in d-wave altermagnetic V2Se2O crystals.
- Explore the influence of dimensionality and K-intercalation on spin dynamics.
Main Methods:
- Utilized real-time time-dependent density functional theory (RT-TDDFT).
- Analyzed laser polarization effects on momentum-dependent spin transfer.
- Compared K-intercalated and deintercalated V2Se2O systems.
Main Results:
- Laser polarization selectively excites momentum-dependent spin transfer in V2Se2O.
- Anisotropic optical intersite spin transfer generates transient net magnetization.
- Deintercalated and monolayer V2Se2O show significantly larger laser-induced magnetization than K-intercalated bulk.
Conclusions:
- Dimensionality and K-intercalation are key factors in tailoring ultrafast spin responses.
- Altermagnets like V2Se2O are promising for ultrafast spintronic applications.
- K-intercalation suppresses spin-relaxation channels, enhancing laser-induced magnetization.
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