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Nickel Cluster-Based Organic Framework-Functionalized Solid-State Electrolyte for Lithium-Metal Batteries.

Changqi Gu1, Wenyu Ding1, Hongbo Tai1

  • 1College of Chemistry and Chemical Engineering, Inner Mongolia University, Hohhot 010021, P. R. China.

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|April 2, 2026
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Summary
This summary is machine-generated.

Researchers developed a novel lithium-metal battery solid-state electrolyte, Ni-MOF-OLi-1, using modified metal-organic frameworks. This new material significantly enhances ionic conductivity and capacity retention for safer, more efficient batteries.

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Area of Science:

  • Materials Science
  • Electrochemistry
  • Energy Storage

Background:

  • Low ionic conductivity and poor capacity retention limit solid-state electrolytes (SSEs) in lithium-metal batteries (LMBs).
  • Metal-organic frameworks (MOFs) offer potential for developing advanced SSEs due to their tunable structures.

Purpose of the Study:

  • To synthesize and characterize novel trinuclear cluster-based MOFs modified with LiOH for improved SSE performance.
  • To evaluate the electrochemical properties of the modified MOF (Ni-MOF-OLi-1) for application in lithium-metal batteries.

Main Methods:

  • Synthesis of Ni-MOF-OH and its subsequent modification with LiOH to form Ni-MOF-OLi-1.
  • Electrochemical characterization including ionic conductivity (σ), electrochemical stability window, and Li+ transference number measurements.
  • Assembly and testing of a LiFePO4 (LFP)/Li battery cell using the developed SSE.

Main Results:

  • Ni-MOF-OLi-1 exhibited a higher ionic conductivity (1.55 × 10⁻³ S cm⁻¹) and wider electrochemical stability window (5.3 V) compared to Ni-MOF-OH.
  • Excellent ionic conductivity was maintained across a wide temperature range (-40 to 100 °C) with low activation energy (0.09 eV).
  • The LFP/Li cell with Ni-MOF-OLi-1 achieved outstanding capacity retention of 96.33% after 150 cycles.

Conclusions:

  • The LiOH-modified MOF, Ni-MOF-OLi-1, significantly enhances electrochemical performance for solid-state electrolytes.
  • This work presents a promising strategy for developing high-performance SSEs for advanced lithium-metal batteries.