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Related Concept Videos

The Electrical Double Layer01:30

The Electrical Double Layer

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In the region where two bulk phases meet, an intricate electric charge distribution arises due to charge transfer, ion adsorption, molecular orientation, and charge distortion. This complex distribution is commonly referred to as the electrical double layer.When a solid electrode interfaces with ions in an electrolyte solution, the speed of electron transfer dictates the rates of oxidation and reduction. The electrode acquires a charge through the escape of atoms into the solution as cations or...
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Theory of Strong Electrolytes01:23

Theory of Strong Electrolytes

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The interionic forces of the strong electrolytes depend on the solvent's dielectric constant, which is the ability of a solvent to store electrical energy, based on its polarizability. and the solution's concentration. In high-dielectric solvents and in dilute solutions, weak electrostatic forces keep ions apart. However, in low-dielectric solvents or concentrated solutions, stronger interionic forces may cause ions to pair up as ionic doublets despite being fully ionized. The theory of strong...
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Intermolecular Forces03:13

Intermolecular Forces

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Atoms and molecules interact through bonds (or forces): intramolecular and intermolecular. The forces are electrostatic as they arise from interactions (attractive or repulsive) between charged species (permanent, partial, or temporary charges) and exist with varying strengths between ions, polar, nonpolar, and neutral molecules. The different types of intermolecular forces are ion–dipole, dipole–dipole, hydrogen bonds, and dispersion; among these, dipole–dipole, hydrogen...
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Interfacial Electrochemical Methods: Overview01:06

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Interfacial electrochemical methods focus on the phenomena occurring at the boundary between an electrode and a solution, as opposed to bulk methods that concentrate on the solution's overall properties. These interfacial methods are classified as either static or dynamic based on the presence of a nonzero current in the electrochemical cell and the consistency of analyte concentrations. Static methods, such as potentiometry, measure the cell's potential without any significant current...
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Ionic Bonding and Electron Transfer02:48

Ionic Bonding and Electron Transfer

46.7K
Ions are atoms or molecules bearing an electrical charge. A cation (a positive ion) forms when a neutral atom loses one or more electrons from its valence shell, and an anion (a negative ion) forms when a neutral atom gains one or more electrons in its valence shell. Compounds composed of ions are called ionic compounds (or salts), and their constituent ions are held together by ionic bonds: electrostatic forces of attraction between oppositely charged cations and anions. 
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Ionic Bonds00:42

Ionic Bonds

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Overview
When atoms gain or lose electrons to achieve a more stable electron configuration they form ions. Ionic bonds are electrostatic attractions between ions with opposite charges. Ionic compounds are rigid and brittle when solid and may dissociate into their constituent ions in water. Covalent compounds, by contrast, remain intact unless a chemical reaction breaks them.
Opposing Charges Hold Ions Together in Ionic Compounds
Ionic bonds are reversible electrostatic interactions between ions...
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Interlayer-Driven Interfacial Stabilization in Solid Electrolytes for Lithium Batteries: Promises and Challenges.

Madan Bahadur Saud1, Hansheng Li1, M Bilal Faheem1

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Summary
This summary is machine-generated.

Interlayer engineering is crucial for stabilizing solid-state batteries. Functional interlayers improve performance and safety in high-energy solid-state Li-metal batteries by addressing interfacial issues.

Keywords:
anode‐electrolyte interfacecathode‐electrolyte interfaceinterfacial engineeringinterlayer engineeringsolid electrolytessolid‐state batteries

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Area of Science:

  • Materials Science
  • Electrochemistry
  • Energy Storage

Background:

  • Solid-state Li-metal batteries (ASSLBs) offer high energy density but face challenges from interfacial impedance.
  • Sulfide and halide solid electrolytes (SEs) show promise due to high conductivity and mechanical properties.
  • Interfacial instability between SEs and electrodes hinders practical ASSLB applications.

Purpose of the Study:

  • To review recent advancements in interlayer engineering for sulfide and halide SEs in ASSLBs.
  • To establish design principles for interlayers balancing electrochemical stability, ion transport, and mechanical compliance.
  • To identify future research directions for scalable interlayer engineering in high-performance ASSLBs.

Main Methods:

  • Literature review of interlayer engineering strategies for sulfide and halide solid electrolytes.
  • Analysis of interfacial phenomena and their impact on ASSLB performance.
  • Synthesis of design principles for optimizing interlayer functionality.

Main Results:

  • Interlayer engineering effectively suppresses electrolyte decomposition and stabilizes interphases.
  • Functional interlayers reduce space-charge effects and homogenize Li flux.
  • Optimized interlayers enhance electrochemical stability and ion transport in ASSLBs.

Conclusions:

  • Interlayer engineering is a key strategy for overcoming interfacial challenges in ASSLBs.
  • Unified design principles are emerging for developing robust and efficient interlayers.
  • Further research is needed for scalable interlayer solutions to accelerate ASSLB commercialization.