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Related Concept Videos

Batteries and Fuel Cells03:12

Batteries and Fuel Cells

A battery is a galvanic cell that is used as a source of electrical power for specific applications. Modern batteries exist in a multitude of forms to accommodate various applications, from tiny button batteries such as those that power wristwatches to the very large batteries used to supply backup energy to municipal power grids. Some batteries are designed for single-use applications and cannot be recharged (primary cells), while others are based on conveniently reversible cell reactions that...
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Updated: Jun 3, 2026

Construction and Testing of Coin Cells of Lithium Ion Batteries
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Published on: August 2, 2012

Anode-Free All-Solid-State Batteries: Understanding Limitations and Charting a Path to Enhanced Performance.

Sion Kim1, Jaechan Lee1, Jihyun Jang2

  • 1Department of Chemistry, Sogang University, Seoul, Republic of Korea.

Small (Weinheim an Der Bergstrasse, Germany)
|June 2, 2026
PubMed
Summary
This summary is machine-generated.

Anode-free all-solid-state batteries offer high energy density but face interfacial instability due to direct lithium plating. Addressing chemical, thermal, electrochemical, and mechanical vulnerabilities is crucial for their commercial viability.

Keywords:
all‐solid‐state batteriesanode‐freecell assembly and conditionsinterlayer engineeringpressure‐regulating buffer layerssacrificial cathodessolid‐state electrolyte modificationsulfide‐based solid‐state electrolyte

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Characterization of Electrode Materials for Lithium Ion and Sodium Ion Batteries Using Synchrotron Radiation Techniques
10:03

Characterization of Electrode Materials for Lithium Ion and Sodium Ion Batteries Using Synchrotron Radiation Techniques

Published on: November 11, 2013

Area of Science:

  • Materials Science
  • Electrochemistry
  • Energy Storage

Background:

  • All-solid-state batteries (ASSBs) with sulfide solid-state electrolytes (SSEs) are promising for high-energy-density systems.
  • Anode-free ASSBs, utilizing direct lithium (Li) plating, aim to maximize energy density but suffer from interfacial instability.

Purpose of the Study:

  • To review the chemical, thermal, electrochemical, and mechanical vulnerabilities of anode-free sulfide ASSBs.
  • To identify challenges hindering the commercial viability of these advanced battery systems.

Main Methods:

  • Comprehensive analysis of existing literature on anode-free sulfide ASSBs.
  • Examination of interfacial phenomena between SSEs and current collectors.
  • Evaluation of degradation mechanisms under various conditions (chemical, thermal, electrochemical, mechanical).

Main Results:

  • Atmospheric exposure leads to toxic H2S gas and current collector corrosion.
  • A narrow electrochemical stability window promotes the formation of an unstable SEI-like layer, causing Li dendrite growth.
  • Non-uniform Li plating/stripping, dead Li accumulation, inadequate pressure, and volume changes degrade cycling stability.

Conclusions:

  • Sophisticated interfacial engineering strategies are essential to mitigate degradation.
  • Active pressure management systems are needed to accommodate volume variations during cycling.
  • Overcoming these challenges is critical for the successful commercialization of anode-free sulfide ASSBs.