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In Situ Neutron Powder Diffraction Using Custom-made Lithium-ion Batteries
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Published on: November 10, 2014

Quantifying the Absolute Mechanical Baseline of Lithium Plating via First-Principles Assisted Operando Expansion

Junkang Xu1, Xingmin He1, Jiangfeng Huang1

  • 1Department of Thermal Science and Energy Engineering, University of Science and Technology of China, Hefei, Anhui 230026, China.

Nano Letters
|June 25, 2026
PubMed
Summary
This summary is machine-generated.

This study establishes a physical baseline for detecting lithium plating in fast-charging lithium-ion batteries. This breakthrough enables early detection, preventing dendrite growth and improving battery safety.

Keywords:
First-principles calculationsIn situ mechanical diagnosticsLithium platingMechano-electrochemical couplingQuantitative criterion

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Area of Science:

  • Materials Science
  • Electrochemistry
  • Battery Technology

Background:

  • Fast charging in lithium-ion batteries is limited by lithium plating.
  • Current detection methods lack a fundamental physical boundary.
  • Macroscopic expansion tracking is a promising but empirically limited tool.

Purpose of the Study:

  • To establish an absolute mechanical baseline for lithium plating detection.
  • To quantitatively decouple intercalation strain from metallic deposition volume.
  • To develop a robust diagnostic for early lithium plating detection.

Main Methods:

  • Bridging first-principles calculations with operando tracking.
  • Quantitative decoupling of volumetric strain components.
  • Experimental validation using pouch-cell platforms.

Main Results:

  • A rigorous theoretical threshold of 1.20 × 10-4 cm3/C for lithium plating was established.
  • The baseline accurately captured mechanical anomalies during lithium nucleation.
  • The diagnostic proved robust under various challenging conditions (overcharge, subzero temperatures, high rates).

Conclusions:

  • The developed physical boundary provides a fundamental threshold for lithium plating.
  • This diagnostic enables millisecond-level current derating for enhanced battery safety.
  • The framework successfully mitigates dendrite growth and promotes dead lithium reintercalation.