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Boosting electrocatalytic nitrate reduction to ammonia through B-site Ni tuning of a triple-conducting perovskite
Sanzhao Song1,2, Mujia Sun3, Obeylaw Moyo3
1School of Green and Low-Carbon Engineering, Yancheng Teachers University, Yancheng, 224007, China. songsz@yctu.edu.cn.
Abstract:
Developing efficient electrocatalysts for nitrate reduction to ammonia remains challenging. Herein, a Ni-modified triple-conducting Ba(Fe0.4Co0.4Zr0.1Y0.1)0.95Ni0.05O3-δ perovskite achieves a high NH3 yield, 98.7% faradaic efficiency, and excellent durability by accelerating the hydrogenation of reaction intermediates during the NO3RR.
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