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Updated: Oct 28, 2026

Quantification of Hydrogen Concentrations in Surface and Interface Layers and Bulk Materials through Depth Profiling with Nuclear Reaction Analysis
Published on: March 29, 2016
Experimental relative axial neutron-field mapping in the Argonauta research reactor using dysprosium activation and
Rogerio Chaffin Nunes1, Gláucia de Oliveira Barreto1, Maria de Lourdes Moreira1
1Serviço de Desenvolvimento de Técnicas Nucleares, Instituto de Engenharia Nuclear, Comissão Nacional de Energia Nuclear (SEDTN/IEN/CNEN), Rio de Janeiro, RJ, 21941-906, Brazil.
Abstract:
Knowledge of spatial variations in the neutron field is required for irradiation planning, reactor characterization, and experimental validation. This work determined the relative axial neutron-field response in fuel element No. 6 of the Argonauta Research Reactor using thirteen 10 wt% Dy-Al wires. The monitors were irradiated simultaneously in a single 30 min run at 340 W between fuel plates 2 and 3. The net areas of the 94.7 keV gamma-ray peak from 165Dy were measured with an HPGe detector and corrected for decay during counting and between the end of irradiation and counting. End-of-irradiation activities were obtained using the full-energy peak efficiency and gamma-ray emission probability, and specific activities were calculated using the total Dy-Al wire mass. The specific activities ranged from 8.45 × 107 to 1.51 × 108 Bq g-1, with the maximum response at 34 cm from the top of the fuel element. The normalized profile showed a broad central maximum and decreasing responses toward both ends. Comparison with an adjusted one-dimensional diffusion reference yielded R2 = 0.960 and RMSE = 0.0298, whereas comparison with a published MCNPX thermal profile for the same fuel element yielded R2 = 0.888 and RMSE = 0.0501. Because cadmium-covered monitors were not used, thermal and epithermal contributions could not be separated; therefore, the results are interpreted as a relative response to the incident neutron field rather than an absolute thermal-neutron flux measurement.
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