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Macroscale Conjugated Microporous Polymers: Controlling Versatile Functionalities Over Several Dimensions.

Weiyi Zhang1, Hongyu Zuo1, Zhonghua Cheng1

  • 1State Key Laboratory for Modification of Chemical Fibers and Polymer Materials, College of Materials Science and Engineering, Donghua University, Shanghai, 201620, China.

Advanced Materials (Deerfield Beach, Fla.)
|February 19, 2022
PubMed
Summary
This summary is machine-generated.

Conjugated microporous polymers (CMPs) are versatile but difficult to process. New fabrication methods create macroscale CMP structures, improving their use in advanced applications like filtration and catalysis.

Keywords:
adsorption and separationenergy storage and conversionheterogeneous catalysismacroscale conjugated microporous polymerssmart materials

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Area of Science:

  • Materials Science
  • Polymer Chemistry

Background:

  • Conjugated microporous polymers (CMPs) offer diverse applications due to their microporous nature.
  • Insolubility and poor processability of CMP powders limit their practical use in devices.
  • Controlling CMP structure at both micro- and macroscales is crucial for expanded applications.

Purpose of the Study:

  • To review recent advances in fabricating CMPs into macroscale structures.
  • To discuss fabrication techniques and the impact of macroscale morphology on CMP properties and applications.
  • To highlight new chemical and physical phenomena arising from macroscale CMP architectures.

Main Methods:

  • Survey of bottom-up synthesis strategies for CMPs.
  • Analysis of fabrication techniques yielding CMPs as films, membranes, aerogels, and sponges.
  • Review of structure-property relationships in macroscale CMPs.

Main Results:

  • Various bottom-up strategies enable CMPs to be formed as films or hybrid materials.
  • Macroscale CMP architectures include membranes, films, aerogels, and sponges.
  • Macroscale morphology influences chemistry and physics, enabling new functionalities.

Conclusions:

  • Fabrication of macroscale CMP structures overcomes traditional processing limitations.
  • Macroscale CMPs show promise in molecular separation, energy storage, catalysis, and sensing.
  • Advances in CMP fabrication open new avenues for material design and application.