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Bound-States-in-the-Continuum-Induced Directional Photoluminescence with Polarization Singularity in WS2 Monolayers.
Jihae Lee1, Minsu Jeong2, Jaehyuck Jang1,3
1Department of Chemical Engineering, Pohang University of Science and Technology (POSTECH), Pohang 37673, Republic of Korea.
Nano Letters
|January 6, 2025
Summary
Researchers controlled the polarization of light emitted by atomically thin tungsten disulfide. This breakthrough enhances light emission intensity and directionality, paving the way for advanced optoelectronic and quantum devices.
Area of Science:
- Materials Science
- Optoelectronics
- Quantum Photonics
Background:
- Monolayer transition metal dichalcogenides (TMDs) are atomically thin materials with direct bandgaps, crucial for optics and optoelectronics.
- However, their room-temperature photoluminescence is randomly polarized, omnidirectional, and weak, hindering practical applications.
Purpose of the Study:
- To achieve spatial control of photoluminescence polarization in monolayer TMDs.
- To enhance the intensity and directionality of photoluminescence for improved device performance.
Main Methods:
- Coupling monolayer tungsten disulfide (WS2) with photonic bands featuring bound states in the continuum (BICs).
- Designing a dielectric photonic crystal slab with BICs that spectrally align with WS2 excitonic resonance.
Main Results:
- Demonstrated spatial control over photoluminescence polarization.
- Modulated emission directionality and enhanced photoluminescence intensity through BIC coupling.
- Achieved improved light extraction and excitation efficiency.
Conclusions:
- Integration of WS2 with BIC-enhanced photonic crystals enables controlled light emission.
- This approach overcomes limitations of random polarization and weak emission in TMDs.
- Facilitates the development of compact, on-chip optoelectronic and quantum photonic devices.

