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Research Advances in Rare-Earth-Based Solid Electrolytes for All-Solid-State Batteries.

Shanshan Song1, Fei He1, Qing Xia2

  • 1Key Laboratory of Superlight Materials and Surface Technology, Ministry of Education, College of Materials Science and Chemical Engineering, Harbin Engineering University, Harbin, 150001, P. R. China.

Small (Weinheim an Der Bergstrasse, Germany)
|April 24, 2025
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Summary
This summary is machine-generated.

Rare earth elements enhance solid-state electrolytes (SSE) for all-solid-state batteries (ASSBs), improving ionic conductivity and stability. This review explores rare-earth-based SSEs for advanced energy storage solutions.

Keywords:
all‐solid‐state batteriesmaterials designrare earth elementssolid electrolytes

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Area of Science:

  • Materials Science
  • Electrochemistry
  • Energy Storage

Background:

  • All-solid-state batteries (ASSBs) and solid-state electrolytes (SSE) are promising alternatives to conventional lithium-ion batteries.
  • Rare earth elements (REEs) incorporation in SSEs significantly advances ionic conductivity, electrochemical stability, and cycle performance.
  • REEs' unique electronic structures and ionic radii are key to their beneficial properties in electrolytes.

Purpose of the Study:

  • To provide a comprehensive review of rare-earth-based solid electrolytes for ASSBs.
  • To investigate the characteristics, applications, modification strategies, and mechanisms of these advanced SSE materials.
  • To offer insights for designing future SSE materials and improving ASSB performance.

Main Methods:

  • Literature review of rare-earth-based oxide, sulfide, halide, and composite polymer solid electrolytes.
  • Analysis of material properties, including ionic conductivity, electrochemical stability, and mechanical strength.
  • Systematic exploration of performance enhancement solutions and ion transport mechanisms in ASSBs.

Main Results:

  • Rare-earth-based SSEs exhibit superior ionic conductivity and electrochemical stability compared to conventional materials.
  • Diverse rare-earth-based SSE types (oxide, sulfide, halide, composite polymer) show significant potential for ASSBs.
  • Understanding of REEs' influence on ion transmission and material properties is crucial for performance optimization.

Conclusions:

  • Rare-earth-based solid electrolytes are critical for developing high-performance all-solid-state batteries.
  • Further research into modification methods and optimization strategies will unlock the full potential of these materials.
  • Future development prospects point towards advanced ASSBs with enhanced safety and energy density.