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Surface-chemistry-controlled growth of NiBDC on carbon nanotubes governs urea oxidation activity
Danjie Meng1,2, Jian Luo2, Lin Tao3
1School of Chemistry and Materials Science, Guizhou Normal University, Guiyang 550025, China.
Abstract:
CNT surface chemistry dictates NiBDC growth and UOR performance. -OH groups preserve the CNT structure and enhance electron transfer; -NH2 triggers carbothermal reduction to Ni0, disrupting graphitic order; and pristine CNTs provide weak π-π interactions. The -OH catalyst achieves 10 mA cm-2 at 1.328 V, establishing a key surface-activity relationship.
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