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Updated: Jun 16, 2026

Ultrafast Time-resolved Near-IR Stimulated Raman Measurements of Functional π-conjugate Systems
Published on: February 10, 2020
Line-by-line control of 10-THz-frequency-spacing Raman sidebands
Kanaka Raju Pandiri1, Takayuki Suzuki, Akira Suda
1Department of Applied Physics and Chemistry, University of Electro-Communications, Chofu-Shi, Tokyo, Japan.
Abstract:
We report line-by-line control of a coherent discrete spectrum (Raman sidebands) with a frequency spacing of 10.6 THz that is produced by an adiabatic Raman process. We show that the spectral phase of the Raman sidebands is finely controlled to the target (flat relative-spectral-phase). This is achieved by employing a combination of a spatial phase controller and a spectral interferometer, which are specifically designed for a high-power discrete spectrum. We also show that such spectral-phase control produces a train of Fourier transform limited pulses with an ultrahigh repetition rate of 10.6 THz in the time domain.
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