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Nanofilament Formation and Regeneration During Cu/Al₂O₃ Resistive Memory Switching
William A Hubbard1,2, Alexander Kerelsky1,2, Grant Jasmin1,2
1†Department of Physics and Astronomy, University of California, Los Angeles, California 90095, United States.
Nano Letters
|May 1, 2015
Summary
Researchers visualized conductive bridge random access memory (CBRAM) switching, finding the filament grows backward toward the source electrode. This clarifies CBRAM operation and reveals distinct growth phases during switching.
Area of Science:
- Materials Science
- Solid-State Physics
- Nanotechnology
Background:
- Conductive bridge random access memory (CBRAM) is a promising alternative to flash memory.
- Understanding the filament switching mechanism is crucial for CBRAM implementation.
- Direct imaging of the nanoscale switching region is challenging due to device encapsulation.
Purpose of the Study:
- To investigate the filament growth direction in Pt/Al2O3/Cu CBRAM devices.
- To elucidate the real-time physics governing the CBRAM switching process.
- To provide direct visual evidence supporting the electrochemical metallization model.
Main Methods:
- Utilized time-resolved scanning transmission electron microscopy (STEM) for high-resolution imaging.
- Employed a realistic device topology for Pt/Al2O3/Cu CBRAM.
- Observed multiple switching cycles across different devices.
Main Results:
- Demonstrated backward filament growth toward the source metal electrode.
- Identified distinct nucleation-limited and potential-limited no-growth periods.
- Visualized subfemtoampere ionic currents preceding nanoampere electronic currents during switching.
Conclusions:
- The observed backward filament growth validates the electrochemical metallization model for CBRAM.
- Time-resolved STEM imaging provides unprecedented insight into CBRAM switching dynamics.
- Understanding ionic and electronic current interplay is key to optimizing CBRAM performance.

