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Updated: Jul 6, 2026

Fabrication of Gate-tunable Graphene Devices for Scanning Tunneling Microscopy Studies with Coulomb Impurities
Published on: July 24, 2015
Hyperfine interactions in graphene and related carbon nanostructures
1Ecole Polytechnique Fédérale de Lausanne, Institute of Chemical Sciences and Engineering and Institute of Theoretical Physics, CH-1015 Lausanne, Switzerland. oleg.yazyev@epfl.ch
Hyperfine interactions in graphene nanostructures are analyzed. Understanding these magnetic interactions enables the design of carbon nanostructures for advanced spintronics and quantum computing applications.
Area of Science:
- Condensed Matter Physics
- Materials Science
- Quantum Chemistry
Background:
- Hyperfine interactions are crucial for electron spin manipulation in nanomaterials.
- Graphene and carbon nanostructures are promising for spintronics and quantum information processing.
- Understanding these interactions is key to improving spin coherence times.
Purpose of the Study:
- To investigate hyperfine interactions in graphene and related carbon nanostructures.
- To establish a method for accurately describing these interactions.
- To provide parameters for designing improved carbon-based nanodevices.
Main Methods:
- First principles calculations on graphene fragments.
- Statistical analysis of interaction parameters.
- Determination of hyperfine interaction parameters for 13C and other nuclear spins.
Main Results:
- Both isotropic and dipolar hyperfine interactions in sp2 carbon nanostructures are accurately described by local electron spin distribution and atomic structure.
- A comprehensive set of parameters for hyperfine interactions at impurities and edges was determined.
- The findings facilitate the design of nanostructures with enhanced electron spin coherence.
Conclusions:
- The study provides a framework for understanding and controlling hyperfine interactions in carbon nanostructures.
- Results enable the development of graphene-based materials for spintronics and quantum computing.
- Practical guidelines for minimizing hyperfine interactions are presented.
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